Volume 10 Issue 4
Jul.  2020
Turn off MathJax
Article Contents
Article Navigation >  Journal of Environmental Engineering Technology  > 2020  >  10(4): 647-652
WANG Zhichao, HE Jie, ZHANG Manli, CAI Hongying, HUANG Zechun. Release characteristics of PAHs in oil-based drilling cuttings solidified body[J]. Journal of Environmental Engineering Technology, 2020, 10(4): 647-652. doi: 10.12153/j.issn.1674-991X.20200013
Citation: WANG Zhichao, HE Jie, ZHANG Manli, CAI Hongying, HUANG Zechun. Release characteristics of PAHs in oil-based drilling cuttings solidified body[J]. Journal of Environmental Engineering Technology, 2020, 10(4): 647-652. doi: 10.12153/j.issn.1674-991X.20200013
shu

Release characteristics of PAHs in oil-based drilling cuttings solidified body

doi: 10.12153/j.issn.1674-991X.20200013
  • 1.

    Chinese Research Academy of Environmental Sciences

  • 2.

    Chongqing Solid Waste Management Center

More Information
  • Corresponding author: HUANG Zechun E-mail: huangzc@craes.org.cn
  • Received Date: 2020-02-09
  • Publish Date: 2020-07-20
    Abstract
  • An effective way to further dispose and utilize resources is to make oil-based drilling cuttings into blocky solidified body. However, when solidified body is used, PAHs may leach out. The release characteristics of 5 kinds of polycyclic aromatic hydrocarbons (PAHs) in solidified body, including naphthalene, anthracene, fluoranthene, benzo (b) fluoranthene and benzo (a) pyrene (BaP), were studied by using the test method of effective amount of inorganic components in solid (NEN7371) and the diffusion test method of inorganic components in bulk materials (NEN7375) and to assess their leaching release risks. The results showed that the effective release rates of the 5 kinds of PAHs were all below 2%. The effective release amount of BaP exceeded the limiting value of Category Ⅲ in Groundwater Quality Standard (GB/T 14848-2017). In static immersion release characteristic experiments, 5 kinds of PAHs released at the early stage, and their accumulated release amount at the previous 16 days accounted for more than 78% of the cumulative total release amount of 64 days. The release mechanism of the 5 kinds of PAHs included diffusion control, dissolution release, delayed release, depletion and surface wash-off. Different PAHs in solidified body had different release characteristics, but in general, they were mainly released in the way of diffusion control. In the later stage, they mainly released in the form of depletion mechanism.

     

    • FullText(HTML)
  • loading
    • References(29)
  • [1]
    张曼丽, 蔡洪英, 周琼. 重庆开展页岩气开采固体废物污染控制研究[J]. 资源再生, 2018(11):42-44.

    ZHANG M L, CAI H Y, ZHOU Q. Research on pollution control of solid waste in shale gas mining in Chongqing[J]. Resource Recycling, 2018(11):42-44.
    [2]
    沈晓莉, 杨金忠, 徐天有, 等. 典型地区油气田水基钻井岩屑污染特征研究[J]. 环境污染与防治, 2017,39(5):480-483.

    SHEN X L, YANG J Z, XU T Y, et al. Research on pollution characteristic of water-based drilling cuttings of typical oil-gas fields[J]. Environmental Pollution & Control, 2017,39(5):480-483.
    [3]
    吴娜, 聂志强, 李开环, 等. 页岩气开采钻井固体废物的污染特性[J]. 中国环境科学, 2019,39(3):1094-1100.

    WU N, NIE Z Q, LI K H, et al. Pollution characteristics of solid waste in shale gas mining drilling[J]. China Environmental Science, 2019,39(3):1094-1100.
    [4]
    KOGBARA R B, DUMKHANA B B, AYOTAMUNO J M, et al. Recycling stabilised/solidified drill cuttings for forage production in acidic soils[J]. Chemosphere, 2017,184:652-663.
    doi: 10.1016/j.chemosphere.2017.06.042 pmid: 28628902
    [5]
    ZHANG X Y, YAO A G. Pilot experiment of oily cuttings thermal desorption and heating characteristics study[J]. Journal of Petroleum Exploration and Production Technology, 2018,16:1-8.
    [6]
    CHEN J, YAN L, WAN X L. The environmental protection problems in drilling a well[J]. Safety and Environmental Engineering, 2003,10(2):43-44.
    [7]
    YAN P, LU M, GUAN Y, et al. Remediation of oil-based drill cuttings through a biosurfactant-based washing followed by a biodegradation treatment[J]. Bioresoure Technology, 2011,102(22):10252-10259.
    doi: 10.1016/j.biortech.2011.08.074
    [8]
    郭沫. 油气田钻井废弃泥浆固化处理技术的探讨[J]. 中国石油和化工标准与质量, 2018,38(16):156-157.
    [9]
    王朝强, 梅绪东, 何敏, 等. 我国页岩气油基钻屑处理及其资源化利用前景[J]. 粉煤灰综合利用, 2017(5):57-60.

    WANG C Q, MEI X D, HE M, et al. Oil-based drilling cuttings and resource utilization frontier on shale gas in our country[J]. Fly Ash Comprehensive Utilization, 2017(5):57-60.
    [10]
    陆林峰. 钻井固体废物制免烧砖技术及应用[J]. 四川环境, 2012,31(增刊1):68-72.

    LU L F. The application and technology of unburned bricks manufactured by using drilling solid waste[J]. Sichuan Environment, 2012,31(Suppl 1):68-72.
    [11]
    WANG C Q, LIN X Y, MEI X D, et al. Performance of non-fired bricks containing oil-based drilling cuttings pyrolysis residues of shale gas[J]. Cleaner Production, 2019,206:282-296.
    doi: 10.1016/j.jclepro.2018.09.128
    [12]
    ASADI S, MOSTAVI E, UGOCHUKWU E. Feasibility study of the potential use of drill cuttings in concrete[J]. Pavement Research and Technology, 2015,8(6):440-445.
    [13]
    TUNCAN A, TUNCAN M, KOYUNCU H. Use of petroleum contaminated drilling wastes as sub-base material for road construction[J]. Waste Management & Research, 2000,18(5):489-505.
    [14]
    白鹤, 翁良宇, 赵广宇, 等. 钻井岩屑除油技术进展[J]. 当代化工, 2018,47(1):182-186.

    BAI H, WENG L Y, ZHAO G Y, et al. Review of oil removal technology of drill cuttings[J]. Contemporary Chemical Industry, 2018,47(1):182-186.
    [15]
    李开环. 涪陵地区页岩气开采固体废物污染特性及资源化环境风险研究[D]. 重庆:重庆交通大学, 2018.
    [16]
    环境保护部. 地表水环境质量标准:GB 3838—2002[S]. 北京:中国环境科学出版社, 2002.
    [17]
    ABDEL-SHAFY H I, MANSOUR M S M. A review on polycyclic aromatic hydrocarbons:source,environmental impact,effect on human health and remediation[J]. Egyptian Journal of Petroleum, 2016,25(1):107-123.
    doi: 10.1016/j.ejpe.2015.03.011
    [18]
    刘天璐, 杨洁, 王君, 等. 含油污泥及其污染水体中多环芳烃及其急性生物毒性测定[J]. 环境工程学报, 2017,11(5):3051-3058.

    LIU T L, YANG J, WANG J, et al. Determination of polycyclic aromatic hydrocarbons and acute biotoxicty for petroleum sludge and contaminated fresh water[J]. Chinese Journal of Environmental Engineering, 2017,11(5):3051-3058.
    [19]
    KOSSON D S, SLOOT H A V D, SANCHEZ F. An integrated framework for evaluating leaching in waste management and utilization of secondary materials[J]. Environmental Engineering Science, 2002,19(3):159-204.
    doi: 10.1089/109287502760079188
    [20]
    SLOOT H A V D, KOSSON D S. Use of characterisation leaching tests and associated modelling tools in assessing the hazardous nature of wastes[J]. Journal of Hazardous Materials, 2012,207/208:36-43.
    [21]
    Netherlands Normalisation Institute. Leaching characteristics:determination of the availability of inorganic components for leaching-solid earthy and stony materials:NEN7371[S]. Amsterdam:Netherlands Normalisation Institute, 2004.
    [22]
    Netherlands Normalisation Institute. Leaching characteristics:determination of leaching of inorganic components with the diffusion test:NEN7375[S]. Amsterdam:Netherlands Normalisation Institute, 2004.
    [23]
    国土资源部. 地下水质量标准:GB/T 14848—2017[S/OL]. (2017-10-14)[2020-01-20]. http://c.gb688.cn/bzgk/gb/showGb?type=online&hcno=F745E3023BD5B10B9FB5314E0FFB5523.
    [24]
    环境保护部. 土壤和沉积物多环芳烃的测定气相色谱-质谱法:HJ 805—2016[S]. 北京:中国环境科学出版社, 2016.
    [25]
    环境保护部. 水质多环芳烃的测定液液萃取和固相萃取高效液相色谱法:HJ 478—2009[S]. 北京:中国环境科学出版社, 2009.
    [26]
    段华波. 危险废物浸出毒性鉴别理论和方法研究[D]. 北京:中国环境科学研究院, 2006.
    [27]
    SLOOT H A V D. Systematic leaching behaviour of trace elements from construction materials and waste materials[J]. Studies in Environmental Science, 1991,48:19-36.
    [28]
    GHOSH D, GHOSH S, DUTTA T K, et al. Current state of knowledge in microbial degradation of polycyclic aromatic hydrocarbons (PAHs):a review[J]. Frontiers in Microbiology, 2016,7:1369.
    doi: 10.3389/fmicb.2016.01369 pmid: 27630626
    [29]
    张洪梅. 湖泊沉积物中多环芳烃菲吸附解吸特征研究[D]. 南京:南京农业大学, 2014.
    • Relative Articles
    • Supplements(0)
    • Cited By
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF
    XML

    Article Metrics

    Article Views(367) PDF Downloads(91) Cited by()
    Proportional views
    Related

    Copyright © Editorial Department of Journal of Environmental Engineering Technology

    京ICP备05031605号-2

    Supported by: Beijing Renhe Information Technology Co., Ltd.  

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return