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高频介质阻挡放电还原分解CO2气体研究

张凡 王洪昌 石应杰 王红梅 井鹏 任洪岩

张凡, 王洪昌, 石应杰, 王红梅, 井鹏, 任洪岩. 高频介质阻挡放电还原分解CO2气体研究[J]. 环境工程技术学报, 2011, 1(1): 33-37. doi: 10.3969/j.issn.1674-991X.2011.01.006
引用本文: 张凡, 王洪昌, 石应杰, 王红梅, 井鹏, 任洪岩. 高频介质阻挡放电还原分解CO2气体研究[J]. 环境工程技术学报, 2011, 1(1): 33-37. doi: 10.3969/j.issn.1674-991X.2011.01.006
ZHANG Fan, WANG Hong-chang, SHI Ying-jie, WANG Hong-mei, JING Peng, REN Hong-yan. Research on Decomposition of Carbon Dioxide by High Frequency Dielectric Barrier Discharge[J]. Journal of Environmental Engineering Technology, 2011, 1(1): 33-37. doi: 10.3969/j.issn.1674-991X.2011.01.006
Citation: ZHANG Fan, WANG Hong-chang, SHI Ying-jie, WANG Hong-mei, JING Peng, REN Hong-yan. Research on Decomposition of Carbon Dioxide by High Frequency Dielectric Barrier Discharge[J]. Journal of Environmental Engineering Technology, 2011, 1(1): 33-37. doi: 10.3969/j.issn.1674-991X.2011.01.006

高频介质阻挡放电还原分解CO2气体研究

doi: 10.3969/j.issn.1674-991X.2011.01.006
详细信息
    作者简介:

    张凡,男,研究员,硕士,主要从事环境工程研究工作

    通讯作者:

    王洪昌,男,博士后

  • 中图分类号: X701

Research on Decomposition of Carbon Dioxide by High Frequency Dielectric Barrier Discharge

More Information
    Corresponding author: 王洪昌,男,博士后
  • 摘要: 温室效应和全球变暖已成为全球性的环境问题之一,为治理温室气体CO2,采用高频介质阻挡放电等离子体对CO2还原分解进行了研究,考察了放电电压、放电频率、冷却方式和CO2浓度等对CO2分解特性的影响。结果发现:在一定范围内,随着放电电压和放电频率的增大,CO2的转化率增大;通过采用循环水冷或风冷的方式可以降低反应体系的温度,抑制CO2合成副反应的进行,提高CO2的转化率;添加惰性气体降低CO2浓度的方式虽然可以提高CO2转化率,但会造成能量利用效率降低。

     

  • [1] MARCO A L C,DOUGLAS F M G,TAKASHI Y.Optimal resource management control for CO2 emission and reduction of the greenhouse effect[J]. Ecological Modeling,2008,213(1):119-126.
    [2] 高洁,郭斌.温室气体二氧化碳的回收与资源化[J].污染防治技术,2007,20(1):56-59.
    [3] MAEZONO I,CHANG J S.Reduction of CO2 from combustion gases by DC corona torches[J].IEEE Transactions on Industry Applications,1990,26(4):651-655.
    [4] 朱爱民,张秀玲,宫为民,等.常压非平衡等离子体条件下CO2的转化[J].环境科学,1998,19(2):20-23.
    [5] 代斌,宫为民,张秀玲,等.脉冲电晕等离子体活化纯CO2的反应[J].中国环境科学,1999,19(5):410-412.
    [6] 李明伟,许根慧,刘昌俊,等.电晕放电二氧化碳冷等离子体转化特性研究[J].燃料化学学报,2001,29(3):243-246.
    [7] MATSUMOTO H,TANABE S,OKITSU K,et al.Profiles of carbon dioxide decomposition in a Dielectric-Barrier Discharge-Plasma system[J].Bulletin of the Chemical Society of Japan,1999,72(11):2567-2571.
    [8] LI R X,YAMAGUICHI Y,YIN S,et al.Influence of dielectric barrier materials to the behavior of dielectric barrier discharge plasma for CO2 decomposition[J].Solid State Ionics,2004,172(1/4):235-238.
    [9] LI R X,TANG Q,YIN S,et al.Decomposition of carbon dioxide by the Dielectric Barrier Discharge (DBD) Plasma using Ca0.7Sr0.3TiO3 barrier[J].Chemistry Letters,2004,33(4):412-413.
    [10] LI R X,TANG Q,YIN S,et al.Plasma catalysis for CO2 decomposition by using different dielectric materials[J].Fuel Processing Technology,2006,87(7):617-622.
    [11] WANG J Y,XIA G G,HUANG A,et al.CO2 decomposition using glow discharge plasmas[J].Journal of Catalysis,1999,185(1):152-159.
    [12] HSIEH L T,LEE W J,LI C T,et al.Decomposition of carbon dioxide in the RF Plasma environment[J].Journal of Chemistry Technology and Biotechnology,1998,73(4):432-442.
    [13] WEN Y Z,JIANG X Z.Decomposition of CO2 using pulsed corona discharges combined with catalyst[J].Plasma Chemistry and Plasma Processing,2001,21(4):665-678.
    [14] KRAUS M,ELIASSON B,KOGELSCHATZ U,et al.CO2 reforming of methane by the combination of dielectric-barrier discharges and catalysis[J].Physical Chemistry Chemical Physics,2001,3(3):294-300.
    [15] SAVINOV S Y,LEE H,SONG H K,et al.Decomposition of methane and carbon dioxide in a Radio-Frequency Discharge[J].Industrial & Engineering Chemistry Research,1999,38(7):2540-2547.
    [16] LI D H,LI X,BAI M G,et al.CO2 reforming of CH4 by atmospheric pressure glow discharge plasma: a high conversion ability[J].International Journal of Hydrogen Energy,2009,34(1):308-313.
    [17] 谭世语,杨大伟.射频放电等离子体作用下CO2-H2的转化研究[J].天然气化工,2008, 33(5):23-26.
    [18] 许根慧,姜恩永,盛京,等.等离子体技术与应用[M].北京:化学工业出版社,2006.
    [19] TAKAAKI T,KEN K,HIROTAKE K,et al.Carbon materials syntheses using dielectric barrier discharge microplasma in supercritical carbon dioxide environments[J].The Journal of Supercritical Fluids,2007,41(3):404-411.
    [20] JAN S,KRZYSZTOF K,MICHAL M,et al.Plasma-catalytic methane conversion with carbon dioxide in dielectric barrier discharges[J].Applied Catalysis B:Environmental,2010,94(1/2):19-26.
    [21] STEPHANIE L B,TOMOKO S,MANUEL M,et al.Factors influencing the decomposition of CO2 in AC Fan-Type plasma reactors:frequency,waveform and concentration effects[J].Journal of Catalysis,1999,184(1):123-133.
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出版历程
  • 收稿日期:  2010-11-02
  • 修回日期:  2010-11-11
  • 刊出日期:  2011-01-20

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