Volume 13 Issue 3
May  2023
Turn off MathJax
Article Contents
ZHAO X L,DUAN L,ZHOU J L,et al.Distribution characteristics, source analysis and risk assessment of heavy metals in sediments of Wanghu Lake of Hubei Province[J].Journal of Environmental Engineering Technology,2023,13(3):1021-1030 doi: 10.12153/j.issn.1674-991X.20220729
Citation: ZHAO X L,DUAN L,ZHOU J L,et al.Distribution characteristics, source analysis and risk assessment of heavy metals in sediments of Wanghu Lake of Hubei Province[J].Journal of Environmental Engineering Technology,2023,13(3):1021-1030 doi: 10.12153/j.issn.1674-991X.20220729

Distribution characteristics, source analysis and risk assessment of heavy metals in sediments of Wanghu Lake of Hubei Province

doi: 10.12153/j.issn.1674-991X.20220729
  • Received Date: 2022-07-19
  • Accepted Date: 2022-11-28
  • Rev Recd Date: 2022-07-28
  • To reveal the characteristics of heavy metal pollution in the sediments of Wanghu Lake in Hubei Province, the methods of spatial interpolation, principal component analysis, and geo-accumulation index were used to investigate the pollution features, source identification, and ecological risk status of heavy metal pollution. The results showed that the average concentration of five heavy metals decreased in the order of Zn>Cr>Cu>Pb>Cd, and all of them exceeded Hubei soil background values. Pearson correlation analysis revealed a positive correlation (P<0.05) between Zn and Cd, Zn and Pb, and a negative correlation (P<0.05) between Cu and Zn, Cu and Cr. Principal component analysis revealed that principal component 1 was consisted of Pb, Cd, and Zn, which were primarily influenced by river transportation and agricultural activities; principal component 2 was consisted of Cr and Cu, which were mainly affected by natural background such as mineral weathering and pollution from human activities such as industrial activities and aquaculture. The geo-accumulation index results suggested that heavy metals in Wanghu Lake were in a low risk condition, although Cd and Cu reached moderate pollution and were the major pollutants that should be monitored.

     

  • loading
  • [1]
    易雨君, 王文君, 宋劼.长江中下游底泥重金属污染特征、潜在生态风险评价及来源分析[J]. 水利水电技术,2019,50(2):1-7.

    YI Y J, WANG W J, SONG J. Pollution characteristics, potential ecological risk assessment and source analysis of heavy metals of sediment in the middle and lower reaches of the Yangtze River[J]. Water Resources and Hydropower Engineering,2019,50(2):1-7.
    [2]
    唐阵武, 程家丽, 岳勇, 等.武汉典型湖泊沉积物中重金属累积特征及其环境风险[J]. 湖泊科学,2009,21(1):61-68. doi: 10.3321/j.issn:1003-5427.2009.01.008

    TANG Z W, CHENG J L, YUE Y, et al. Accumulations and risks of heavy metals in the sediments from typical lakes in Wuhan, China[J]. Journal of Lake Sciences,2009,21(1):61-68. doi: 10.3321/j.issn:1003-5427.2009.01.008
    [3]
    HU Y, ZHOU J, DU B, et al. Health risks to local residents from the exposure of heavy metals around the largest copper smelter in China[J]. Ecotoxicology and environmental safety,2019,171:329-336. doi: 10.1016/j.ecoenv.2018.12.073
    [4]
    REZAYI M, AHMADZADEH S, KASSIM A, et al. Thermodynamic studies of complex formation between Co (Salen) ionophore with chromate (II) ions in AN-H2O binary solutions by the conductometric method[J]. International Journal of Electrochemical Science,2011,6:6350-6359.
    [5]
    HASEGAWA H, RAHMAN M A, KITAHARA K, et al. Seasonal changes of arsenic speciation in lake waters in relation to eutrophication[J]. Science of the Total Environment,2010,408(7):1684-1690. doi: 10.1016/j.scitotenv.2009.11.062
    [6]
    HU B, LI G, LI J, et al. Spatial distribution and ecotoxicological risk assessment of heavy metals in surface sediments of the southern Bohai Bay, China[J]. Environmental Science and Pollution Research,2013,20(6):4099-4110. doi: 10.1007/s11356-012-1332-z
    [7]
    CHENG H, LI M, ZHAO C, et al. Concentrations of toxic metals and ecological risk assessment for sediments of major freshwater lakes in China[J]. Journal of Geochemical Exploration,2015,157:15-26. doi: 10.1016/j.gexplo.2015.05.010
    [8]
    AGARWAL A, SINGH R D, MISHRA S K, et al. ANN-based sediment yield models for Vamsadhara river basin (India)[J]. Water Sa,2005,31(1):85-100.
    [9]
    MALFERRARI D, BRIGATTI M F, LAURORA A, et al. Heavy metals in sediments from canals for water supplying and drainage: mobilization and control strategies[J]. Journal of Hazardous Materials,2009,161(2/3):723-729. doi: 10.1016/j.jhazmat.2008.04.014
    [10]
    SCHLEISS A J, FRANCA M J, JUEZ C, et al. Reservoir sedimentation[J]. Journal of Hydraulic Research,2016,54(6):595-614. doi: 10.1080/00221686.2016.1225320
    [11]
    余秀娟, 霍守亮, 昝逢宇等.巢湖表层沉积物中砷的分布特征及其污染评价[J]. 环境工程技术学报,2012,2(2):124-132. doi: 10.3969/j.issn.1674-991X.2012.02.019

    YU X J, HUO S L, ZAN F Y, et al. Distribution characteristics and contamination assessment of arsenic in surface sediments of Lake Chaohu, China[J]. Journal of Environmental Engineering Technology,2012,2(2):124-132. doi: 10.3969/j.issn.1674-991X.2012.02.019
    [12]
    RAJESHKUMAR S, LIU Y, ZHANG X, et al. Studies on seasonal pollution of heavy metals in water, sediment, fish and oyster from the Meiliang Bay of Taihu Lake in China[J]. Chemosphere,2018,191:626-638. doi: 10.1016/j.chemosphere.2017.10.078
    [13]
    EKERE N, YAKUBU N, IHEDIOHA J. Ecological risk assessment of heavy metals and polycyclic aromatic hydrocarbons in sediments of rivers Niger and Benue confluence, Lokoja, Central Nigeria[J]. Environmental Science and Pollution Research,2017,24(23):18966-18978. doi: 10.1007/s11356-017-9511-6
    [14]
    CAGNIN R C, QUARESMA V S, CHAILLOU G, et al. Arsenic enrichment in sediment on the eastern continental shelf of Brazil[J]. Science of the Total Environment,2017,607:304-316.
    [15]
    KE X, GUI S, HUANG H, et al. Ecological risk assessment and source identification for heavy metals in surface sediment from the Liaohe River protected area, China[J]. Chemosphere,2017,175:473-481. doi: 10.1016/j.chemosphere.2017.02.029
    [16]
    ZAHRA A, HASHMI M Z, MALIK R N, et al. Enrichment and geo-accumulation of heavy metals and risk assessment of sediments of the Kurang Nallah: feeding tributary of the Rawal Lake Reservoir, Pakistan[J]. Science of the Total Environment,2014,470:925-933.
    [17]
    刘利, 张嘉雯, 陈奋飞, 等.衡水湖底泥重金属污染特征及生态风险评价[J]. 环境工程技术学报,2020,10(2):205-211.

    LIU L, ZHANG J W, CHEN F F, et al. Pollution characteristics and ecological risk assessment of heavy metals in the sediment of Hengshui Lake[J]. Journal of Environmental Engineering Technology,2020,10(2):205-211.
    [18]
    张冬萍, 刘蓬, 刘琳, 等.黄石市磁湖水质时空分布及污染源解析[J]. 环境工程技术学报,2022,12(2):560-566.

    ZHANG D P, LIU P, LIU L, et al. Temporal and spatial distribution of water quality and source apportionment in Cihu Lake, Huangshi City[J]. Journal of Environmental Engineering Technology,2022,12(2):560-566.
    [19]
    周道坤, 刘晓伟, 荣楠, 等.湖北网湖自然保护区水质改善对策研究[J]. 环境科学与技术,2020(增刊2):7.

    ZHOU D K, LIU X W, RONG N, et al. Study on the strategy for the improvement of aquatic quality in Network Lake Wetland Nature Reserve[J]. Environmental Science & Technology,2020(Suppl 2):7.
    [20]
    DIXON B, UDDAMERI V. GIS and geocomputation for water resource science and engineering[M].State of New Jersey: John Wiley & Sons, 2016.
    [21]
    YAN H, SHENGYUAN Y, LI M, et al. Evaluation of heavy metal contamination in agricultural topsoils in suburban Xuchang City, China[J]. Environmental Earth Sciences,2015,74(3):2475-2480. doi: 10.1007/s12665-015-4252-7
    [22]
    MULLER G. Index of geoaccumulation in sediments of the Rhine River[J]. Geojournal,1969,2:108-118.
    [23]
    中国环境监测总站. 中国土壤元素背景值[M]. 北京: 中国环境科学出版社, 1990.
    [24]
    JI Y, ZHANG J, LI R, et al. Distribution and partitioning of heavy metals in sediments of the Xinjiang River in Poyang Lake Region, China[J]. Environmental Progress & Sustainable Energy,2015,34(3):713-723.
    [25]
    史小丽, 秦伯强.长江中游网湖沉积物重金属元素变化特征分析[J]. 第四纪研究,2009(1):9.

    SHI X L, QIN B Q. Analysis on heavy metal distributions in core sediment from Wanghu Lake in the middle reaches of the Yangtze River[J]. Quaternary Sciences,2009(1):9.
    [26]
    鄢明才, 迟清华, 顾铁新, 等. 中国各类沉积物化学元素平均含量[J]. 物探与化探, 1995(6): 468-472.

    YAN M C, CHI Q H, GU T X, et al, Average element content of various sediments in China[J]. Geophysical and Geochemical Exploration, 1995(6): 468-472.
    [27]
    SMITH S L, MACDONALD D D, KEENLEYSIDE K A, et al. A preliminary evaluation of sediment quality assessment values for freshwater ecosystems[J]. Journal of Great Lakes Research,1996,22(3):624-638. doi: 10.1016/S0380-1330(96)70985-1
    [28]
    YAN N, LIU W, XIE H, et al. Distribution and assessment of heavy metals in thesurface sediment of Yellow River, China[J]. Environmental Science & Technology 2016, 39: 45–51.
    [29]
    WANG L, DAI L, LI L, et al. Multivariable cokriging prediction and source analysis of potentially toxic elements (Cr, Cu, Cd, Pb, and Zn) in surface sediments from Dongting Lake, China[J]. Ecological Indicators,2018,94:312-319. doi: 10.1016/j.ecolind.2018.07.005
    [30]
    DAI L, WANG L, LI L, et al. Multivariate geostatistical analysis and source identification of heavy metals in the sediment of Poyang Lake in China[J]. Science of the total environment,2018,621:1433-1444. doi: 10.1016/j.scitotenv.2017.10.085
    [31]
    LIU H Q, ZHANG Y, YUAN Z J, et al. Risk assessment concerning the heavy metals in sediment around Taihu Lake, China[J]. Water Environment Research,2021,93(11):2795-2806. doi: 10.1002/wer.1638
    [32]
    JIANG Q, LIU M, WANG J, et al. Feasibility of using visible and near-infrared reflectance spectroscopy to monitor heavy metal contaminants in urban lake sediment[J]. Catena,2018,162:72-79. doi: 10.1016/j.catena.2017.11.020
    [33]
    高吉权, 朱姗姗, 刘鹏飞.洞庭湖底泥沉积物重金属分布与生态风险评价[J]. 云南大学学报:自然科学版,2019,41(4):851-859.

    GAO J Q, ZHU S S, LIU P F. Spatial distribution characteristics and ecological risk assessment of heavy metals in surface sediments of Dongting Lake[J]. Journal of Yunnan University:Natural Sciences Edition,2019,41(4):851-859.
    [34]
    LI F, HUANG J, ZENG G, et al. Spatial risk assessment and sources identification of heavy metals in surface sediments from the Dongting Lake, Middle China[J]. Journal of Geochemical Exploration,2013,132:75-83. doi: 10.1016/j.gexplo.2013.05.007
    [35]
    史小丽, 秦伯强.长江中游网湖沉积物营养元素变化特征及其影响因素[J]. 地理科学,2010,30(5):766-771.

    SHI X L, QIN B Q. Nutrients distribution character and their influential factors in core sediments from Wanghu Lake in middle reaches of Changjiang River[J]. Scientia Geographica Sinica,2010,30(5):766-771.
    [36]
    史小丽, 秦伯强.长江中游网湖近代沉积环境演变及其对人类活动的响应[J]. 地理研究,2013,32(5):808-816.

    SHI X L, QIN B Q. Environmental evolution of Wanghu Lake in the middle Yangtze River and its responses to human activities[J]. Geographical Research,2013,32(5):808-816.
    [37]
    SONG Y, JI J, YANG Z, et al. Geochemical behavior assessment and apportionment of heavy metal contaminants in the bottom sediments of lower reach of Changjiang River[J]. Catena,2011,85(1):73-81. doi: 10.1016/j.catena.2010.12.009
    [38]
    Tchounwou P B, Yedjou C G, Patlolla A K, et al. Heavy metal toxicity and the environment.[J]. Molecular, Clinical and Environmental Toxicology,2012,101:133–164.
    [39]
    HUANG S, TU J, LIU H, et al. Multivariate analysis of trace element concentrations in atmospheric deposition in the Yangtze River Delta, East China[J]. Atmospheric Environment,2009,43(36):5781-5790. doi: 10.1016/j.atmosenv.2009.07.055
    [40]
    徐艺文. 江汉湖群典型浅水性湖泊水生植物群落多样性研究[D]. 武汉: 湖北大学, 2019.
    [41]
    ATAFAR Z, MESDAGHINIA A, NOURI J, et al. Effect of fertilizer application on soil heavy metal concentration[J]. Environmental Monitoring and Assessment,2010,160(1):83-89.
    [42]
    涂杰峰, 罗钦, 伍云卿, 等.福建水产饲料重金属污染研究[J]. 中国农学通报,2011,27(29):76-79.

    TU J F, LUO Q, WU Y Q, et al. The Study on the heavy metal pollution of aquatic feed in Fujian[J]. Chinese Agricultural Science Bulletin,2011,27(29):76-79.
    [43]
    RINKLEBE J, ANTIĆ-MLADENOVIĆ S, FROHNE T, et al. Nickel in a serpentine-enriched Fluvisol: redox affected dynamics and binding forms[J]. Geoderma,2016,263:203-214. doi: 10.1016/j.geoderma.2015.09.004
    [44]
    DU LAING G, MEERS E, DEWISPELAERE M, et al. Heavy metal mobility in intertidal sediments of the Scheldt estuary: field monitoring[J]. Science of the Total Environment,2009,407(8):2919-2930. doi: 10.1016/j.scitotenv.2008.12.024
    [45]
    MILLER F S, KILMINSTER K L, DEGENS B, et al. Relationship between metals leached and soil type from potential acid sulphate soils under acidic and neutral conditions in Western Australia[J]. Water, Air, and Soil Pollution,2010,205(1):133-147.
    [46]
    毛凌晨, 叶华.氧化还原电位对土壤中重金属环境行为的影响研究进展[J]. 环境科学研究,2018,31(10):1669-1676.

    MAO L C, YE H. Influence of redox potential on heavy metal behavior in soils: a review[J]. Research of Environmental Sciences,2018,31(10):1669-1676. ⊕
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Figures(8)  / Tables(2)

    Article Metrics

    Article Views(175) PDF Downloads(16) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return